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In Naruto Shippuden episode 121, it starts playing at 0:40 or so when Itachi and Kisame are walking together.

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  • welcome to Anime and Manga. the site you linked to is an illegal streaming site as such i have removed the link. in future please use a legal source if you want to link to videos, example sources can be found in this list
    – Memor-X
    Mar 2, 2018 at 0:41

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The song you're referring to is Itachi's theme song. https://www.youtube.com/watch?v=AXLfg2ry_F4

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