Specifically, the rhythm-less, ambient-like theme first appearing in Episode 18 at around the 7:55 mark, when Abarai walks to the holding cells of 6th Squad (plays for around 20 seconds). The same piece appears a few times more, most notably in Episode 55 at around 14:50 mark, when Genryuusai tells Kyoraku and Ukitake that their crimes have gone beyond just a beating (plays for around 30-40 seconds).

I'm pretty sure it's not included in any of the released OSTs, at least not in the first five. Any help in identifying the piece?

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